Item talk:Q247311
From geokb
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"name": "Changes in the chemistry of shallow groundwater related to the 2008 injection of CO2 at the ZERT field site, Bozeman, Montana",
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"abstract": "Approximately 300\u00a0kg/day of food-grade CO2\u00a0was injected through a perforated pipe placed horizontally 2\u20132.3\u00a0m deep during July 9\u2013August 7, 2008 at the MSU-ZERT field test to evaluate atmospheric and near-surface monitoring and detection techniques applicable to the subsurface storage and potential leakage of CO2. As part of this multidisciplinary research project, 80 samples of water were collected from 10 shallow monitoring wells (1.5 or 3.0\u00a0m deep) installed 1\u20136\u00a0m from the injection pipe, at the southwestern end of the slotted section (zone VI), and from two distant monitoring wells. The samples were collected before, during, and following CO2\u00a0injection. The main objective of study was to investigate changes in the concentrations of major, minor, and trace inorganic and organic compounds during and following CO2\u00a0injection. The ultimate goals were (1) to better understand the potential of groundwater quality impacts related to CO2\u00a0leakage from deep storage operations, (2) to develop geochemical tools that could provide early detection of CO2\u00a0intrusion into underground sources of drinking water (USDW), and (3) to test the predictive capabilities of geochemical codes against field data. Field determinations showed rapid and systematic changes in pH (7.0\u20135.6), alkalinity (400\u20131,330\u00a0mg/l as HCO3), and electrical conductance (600\u20131,800\u00a0\u03bcS/cm) following CO2\u00a0injection in samples collected from the 1.5\u00a0m-deep wells. Laboratory results show major increases in the concentrations of Ca (90\u2013240\u00a0mg/l), Mg (25\u201370\u00a0mg/l), Fe (5\u20131,200\u00a0ppb), and Mn (5\u20131,400\u00a0ppb) following CO2\u00a0injection. These chemical changes could provide early detection of CO2\u00a0leakage into shallow groundwater from deep storage operations. Dissolution of observed carbonate minerals and desorption-ion exchange resulting from lowered pH values following CO2\u00a0injection are the likely geochemical processes responsible for the observed increases in the concentrations of solutes; concentrations generally decreased temporarily following four significant precipitation events. The DOC values obtained are 5\u00a0\u00b1\u00a02\u00a0mg/l, and the variations do not correlate with CO2\u00a0injection. CO2\u00a0injection, however, is responsible for detection of BTEX (e.g. benzene, 0\u20130.8\u00a0ppb), mobilization of metals, the lowered pH values, and increases in the concentrations of other solutes in groundwater. The trace metal and BTEX concentrations are all significantly below the maximum contaminant levels (MCLs). Sequential leaching of core samples is being carried out to investigate the source of metals and other solutes.",
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