Item talk:Q303740
From geokb
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"name": "Towards a holistic sulfate-water-O2 triple oxygen isotope systematics",
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"abstract": "Triple\u00a0oxygen isotope\u00a0(\u220617O with \u03b418O) signals of H2O and O2\u00a0found in\u00a0sulfate\u00a0of oxidative weathering origin offer promising constraints on modern and ancient weathering, hydrology,\u00a0atmospheric gas\u00a0concentrations, and bioproductivity. However, interpretations of the sulfate-water-O2\u00a0system rely on assuming fixed oxygen-isotope fractionations between sulfate and water, which, contrastingly, are shown to vary widely in sign and amplitude. Instead, here we anchor sulfate-water-O2\u00a0triple oxygen isotope systematics on the homogeneous composition of atmospheric O2\u00a0with empirical constraints and modeling. Our resulting framework does not require a priori assumptions of the O2- versus H2O\u2011oxygen ratio in sulfate and accounts for the signals of mass-dependent and mass-independent fractionation in the \u220617O and \u03b418O of sulfate's O2\u2011oxygen source. Within this framework, new \u220617O measurements of sulfate constrain ~2.3\u00a0Ga Paleoproterozoic gross primary productivity to between 6 and 160 times present-day levels, with important implications for the biological\u00a0carbon cycle\u00a0response to high CO2\u00a0concentrations prevalent on the early Earth.",
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