Item talk:Q269328
From geokb
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"name": "Most Earth-surface calcites precipitate out of isotopic equilibrium",
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"abstract": "Oxygen-isotope thermometry played a critical role in the rise of modern geochemistry and remains extensively used in (bio-)geoscience. Its theoretical foundations rest on the assumption that\u00a018O/16O partitioning among water and carbonate minerals primarily reflects thermodynamic equilibrium. However, after decades of research, there is no consensus on the true equilibrium\u00a018O/16O fractionation between calcite and water (18\u03b1cc/w). Here, we constrain the equilibrium relations linking temperature,\u00a018\u03b1cc/w, and clumped isotopes (\u039447) based on the composition of extremely slow-growing calcites from Devils Hole and Laghetto Basso (Corchia Cave). Equilibrium\u00a018\u03b1cc/w\u00a0values are systematically ~1.5\u2030 greater than those in biogenic and synthetic calcite traditionally considered to approach oxygen-isotope equilibrium. We further demonstrate that subtle disequilibria also affect\u00a0\u039447\u00a0in biogenic calcite. These observations provide evidence that most Earth-surface calcites fail to achieve isotopic equilibrium, highlighting the need to improve our quantitative understanding of non-equilibrium isotope fractionation effects instead of relying on phenomenological calibrations.",
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