Item talk:Q251203
From geokb
{
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"@type": "Article",
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"name": "Quantifying differences in the impact of variable chemistry on equilibrium uranium(VI) adsorption properties of aquifer sediments",
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"value": "10.1021/es202677v",
"url": "https://doi.org/10.1021/es202677v"
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"name": "Environmental Science & Technology",
"volumeNumber": "45",
"issueNumber": "20"
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"datePublished": "2011",
"dateModified": "2020-01-11",
"abstract": "Uranium adsorption-desorption on sediment samples collected from the Hanford 300-Area, Richland, WA varied extensively over a range of field-relevant chemical conditions, complicating assessment of possible differences in equilibrium adsorption properties. Adsorption equilibrium was achieved in 500-1000 h although dissolved uranium concentrations increased over thousands of hours owing to changes in aqueous chemical composition driven by sediment-water reactions. A nonelectrostatic surface complexation reaction, >SOH + UO22+ + 2CO32- = >SOUO2(CO3HCO3)2-, provided the best fit to experimental data for each sediment sample resulting in a range of conditional equilibrium constants (logKc) from 21.49 to 21.76. Potential differences in uranium adsorption properties could be assessed in plots based on the generalized mass-action expressions yielding linear trends displaced vertically by differences in logKc values. Using this approach, logKc values for seven sediment samples were not significantly different. However, a significant difference in adsorption properties between one sediment sample and the fines (<0.063 mm) of another could be demonstrated despite the fines requiring a different reaction stoichiometry. Estimates of logKc uncertainty were improved by capturing all data points within experimental errors. The mass-action expression plots demonstrate that applying models outside the range of conditions used in model calibration greatly increases potential errors.",
"description": "8 p.",
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"name": "ACS Publications"
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"name": "Kent, Douglas B. dbkent@usgs.gov",
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"name": "Stoliker, Deborah L. dlstoliker@usgs.gov",
"givenName": "Deborah L.",
"familyName": "Stoliker",
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"affiliation": [
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